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dc.contributor.authorGhosh, A.en
dc.contributor.authorJönsson, H. J. M.en
dc.contributor.authorMukkattukavil, D. J.en
dc.contributor.authorKvashnin, Y.en
dc.contributor.authorPhuyal, D.en
dc.contributor.authorThunström, P.en
dc.contributor.authorAgåker, M.en
dc.contributor.authorNicolaou, A.en
dc.contributor.authorJonak, M.en
dc.contributor.authorKlingeler, R.en
dc.contributor.authorKamalakar, M. V.en
dc.contributor.authorSarkar, T.en
dc.contributor.authorVasiliev, A. N.en
dc.contributor.authorButorin, S. M.en
dc.contributor.authorEriksson, O.en
dc.contributor.authorAbdel-Hafiez, M.en
dc.date.accessioned2024-04-05T16:18:33Z-
dc.date.available2024-04-05T16:18:33Z-
dc.date.issued2023-
dc.identifier.citationGhosh, A, Jönsson, HJM, Mukkattukavil, DJ, Kvashnin, Y, Phuyal, D, Thunström, P, Agåker, M, Nicolaou, A, Jonak, M, Klingeler, R, Kamalakar, MV, Sarkar, T, Vasiliev, AN, Butorin, SM, Eriksson, O & Abdel-Hafiez, M 2023, 'Magnetic circular dichroism in the dd excitation in the van der Waals magnet CrI3 probed by resonant inelastic x-ray scattering', Physical Review B, Том. 107, № 11, 115148. https://doi.org/10.1103/PhysRevB.107.115148harvard_pure
dc.identifier.citationGhosh, A., Jönsson, H. J. M., Mukkattukavil, D. J., Kvashnin, Y., Phuyal, D., Thunström, P., Agåker, M., Nicolaou, A., Jonak, M., Klingeler, R., Kamalakar, M. V., Sarkar, T., Vasiliev, A. N., Butorin, S. M., Eriksson, O., & Abdel-Hafiez, M. (2023). Magnetic circular dichroism in the dd excitation in the van der Waals magnet CrI3 probed by resonant inelastic x-ray scattering. Physical Review B, 107(11), [115148]. https://doi.org/10.1103/PhysRevB.107.115148apa_pure
dc.identifier.issn2469-9950-
dc.identifier.otherFinal2
dc.identifier.otherAll Open Access, Hybrid Gold3
dc.identifier.otherhttps://www.scopus.com/inward/record.uri?eid=2-s2.0-85151298553&doi=10.1103%2fPhysRevB.107.115148&partnerID=40&md5=902652cb8f1766ac2d466abe8168ba391
dc.identifier.otherhttp://link.aps.org/pdf/10.1103/PhysRevB.107.115148pdf
dc.identifier.urihttp://elar.urfu.ru/handle/10995/130323-
dc.description.abstractWe report on a combined experimental and theoretical study on CrI3 single crystals by employing the polarization dependence of resonant inelastic x-ray scattering (RIXS). Our investigations reveal multiple Cr 3d orbital splitting (dd excitations) as well as magnetic dichroism (MD) in the RIXS spectra. The dd excitation energies are similar on the two sides of the ferromagnetic transition temperature, TC∼61 K, although MD in RIXS is predominant at 0.4 T magnetic field below TC. This demonstrates that the ferromagnetic superexchange interaction that is responsible for the interatomic exchange field is vanishingly small compared with the local exchange field that comes from exchange and correlation interaction among the interacting Cr 3d orbitals. The recorded RIXS spectra reported here reveal clearly resolved Cr 3d intraorbital dd excitations that represent transitions between electronic levels that are heavily influenced by dynamic correlations and multiconfiguration effects. Our calculations taking into account the Cr 3d hybridization with the ligand valence states and the full multiplet structure due to intra-atomic and crystal field interactions in Oh and D3d symmetry clearly reproduced the dichroic trend in experimental RIXS spectra. © 2023 authors. Published by the American Physical Society. Published by the American Physical Society under the terms of the "https://creativecommons.org/licenses/by/4.0/"Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI. Funded by "https://www.kb.se/samverkan-och-utveckling/oppen-tillgang-och-bibsamkonsortiet/bibsamkonsortiet.html"Bibsam.en
dc.description.sponsorshipEuropean Research Council, ERC: 2019-03569, 854843-FASTCORR; Deutsche Forschungsgemeinschaft, DFG: 101002772-SPINNER, EXC2181/1-390900948; Stiftelsen för Strategisk Forskning, SSF: RIF14-0064; Bundesministerium für Bildung und Forschung, BMBF: 13XP5088; Carl Tryggers Stiftelse för Vetenskaplig Forskning; Göran Gustafssons Stiftelse för Naturvetenskaplig och Medicinsk Forskning: 075-15-2021-604, 2017-05030, 2018-05973, 2020-00681, 2021-03675; Knut och Alice Wallenbergs Stiftelse; Vetenskapsrådet, VR: 2018-05393; Horizon 2020: 824109en
dc.description.sponsorshipThe authors would like to thank Håkan Rensmo for the fruitful discussions. A.G. and M.A.-H. acknowledge financial support from the Carl Tryggers Foundation and the Swedish Research Council (VR) under Project No. 2018-05393. D.J.M. acknowledges support from SSF Grant No. RIF14-0064. O.E. acknowledges financial support from the Knut and Alice Wallenberg Foundation, eSSENCE, the Swedish Research Council (VR), and the Foundation for Strategic Research (SSF). O.E. and P.T. acknowledge support from ERC synergy Grant No. 854843-FASTCORR. Y.K. acknowledges support from VR (Project No. 2019-03569) and the Göran Gustafsson Foundation. Support from the P220 program Project No. 075-15-2021-604 is acknowledged. The computations were enabled by resources provided by the Swedish National Infrastructure for Computing (SNIC) at the National Supercomputer Centre (NSC) partially funded by the Swedish Research Council through Grant Agreement No. 2018-05973. D.P. acknowledges support from the Swedish Research Council under Project No. 2020-00681. T.S. acknowledges financial support from the Swedish Research Council (VR Grants No. 2017-05030 and No. 2021-03675). M.H. acknowledges support by the European Union's Horizon 2020 Research and Innovation Programme, under Grant Agreement No. 824109 (European Microkelvin Platform). Work at Heidelberg has been supported by BMBF via the project SpinFun (13XP5088) and by Deutsche Forschungsgemeinschaft (DFG) under Germany's Excellence Strategy EXC2181/1-390900948 (the Heidelberg STRUCTURES Excellence Cluster). M.V.K. acknowledges support from ERC Grant No. 101002772-SPINNER.en
dc.format.mimetypeapplication/pdfen
dc.language.isoenen
dc.publisherAmerican Physical Societyen
dc.rightsinfo:eu-repo/semantics/openAccessen
dc.rightscc-byother
dc.rights.urihttps://creativecommons.org/licenses/by/4.0/unpaywall
dc.sourcePhysical Review B2
dc.sourcePhysical Review Ben
dc.subjectCHROMIUMen
dc.subjectCRYSTAL ATOMIC STRUCTUREen
dc.subjectCRYSTAL SYMMETRYen
dc.subjectDICHROISMen
dc.subjectFERROMAGNETIC MATERIALSen
dc.subjectFERROMAGNETISMen
dc.subjectSINGLE CRYSTALSen
dc.subjectVAN DER WAALS FORCESen
dc.subjectX RAY SCATTERINGen
dc.subject3D-ORBITAL SPLITTINGen
dc.subjectD-D EXCITATIONSen
dc.subjectEXCHANGE FIELDSen
dc.subjectMAGNETIC CIRCULAR DICHROISMSen
dc.subjectMAGNETIC DICHROISMen
dc.subjectPOLARIZATION DEPENDENCEen
dc.subjectRESONANT INELASTIC X-RAY SCATTERINGen
dc.subjectTHEORETICAL STUDYen
dc.subjectVAN DER WAALen
dc.subjectX-RAY SCATTERING SPECTRAen
dc.subjectCHROMIUM COMPOUNDSen
dc.titleMagnetic circular dichroism in the dd excitation in the van der Waals magnet CrI3 probed by resonant inelastic x-ray scatteringen
dc.typeArticleen
dc.typeinfo:eu-repo/semantics/articleen
dc.type|info:eu-repo/semantics/publishedVersionen
dc.identifier.doi10.1103/PhysRevB.107.115148-
dc.identifier.scopus85151298553-
local.contributor.employeeGhosh, A., Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Sweden, MAX IV Laboratory, Lund University, P.O. Box 118, Lund, SE-22100, Swedenen
local.contributor.employeeJönsson, H.J.M., Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Sweden, Asia Pacific Center for Theoretical Physics, Pohang, 37673, South Koreaen
local.contributor.employeeMukkattukavil, D.J., Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Swedenen
local.contributor.employeeKvashnin, Y., Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Swedenen
local.contributor.employeePhuyal, D., Department of Applied Physics, KTH Royal Institute of Technology, Stockholm, SE-106 91, Swedenen
local.contributor.employeeThunström, P., Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Swedenen
local.contributor.employeeAgåker, M., Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Sweden, MAX IV Laboratory, Lund University, P.O. Box 118, Lund, SE-22100, Swedenen
local.contributor.employeeNicolaou, A., Synchrotron SOLEIL, L'Orme des Merisiers, Saint-Aubin, BP48, Gif-sur-Yvette, F-91192, Franceen
local.contributor.employeeJonak, M., Kirchhoff Institute of Physics, Heidelberg University, Heidelberg, D-69120, Germanyen
local.contributor.employeeKlingeler, R., Kirchhoff Institute of Physics, Heidelberg University, Heidelberg, D-69120, Germanyen
local.contributor.employeeKamalakar, M.V., Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Swedenen
local.contributor.employeeSarkar, T., Department of Materials Science and Engineering, Uppsala University, Box 35, Uppsala, SE-751 03, Swedenen
local.contributor.employeeVasiliev, A.N., National University of Science and Technology MISiS, Moscow, 119049, Russian Federation, Lomonosov Moscow State University, Moscow, 119991, Russian Federation, Ural Federal University, Ekaterinburg, 620002, Russian Federationen
local.contributor.employeeButorin, S.M., Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Swedenen
local.contributor.employeeEriksson, O., Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Sweden, School of Science and Technology, Örebro University, Örebro, SE-701 82, Swedenen
local.contributor.employeeAbdel-Hafiez, M., Department of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Sweden, University of Doha for Science and Technology, P.O. Box 24449, Doha, Qataren
local.issue11-
local.volume107-
dc.identifier.wos000961165700008-
local.contributor.departmentDepartment of Physics and Astronomy, Uppsala University, Box 516, Uppsala, SE-751 20, Swedenen
local.contributor.departmentMAX IV Laboratory, Lund University, P.O. Box 118, Lund, SE-22100, Swedenen
local.contributor.departmentAsia Pacific Center for Theoretical Physics, Pohang, 37673, South Koreaen
local.contributor.departmentDepartment of Applied Physics, KTH Royal Institute of Technology, Stockholm, SE-106 91, Swedenen
local.contributor.departmentSynchrotron SOLEIL, L'Orme des Merisiers, Saint-Aubin, BP48, Gif-sur-Yvette, F-91192, Franceen
local.contributor.departmentKirchhoff Institute of Physics, Heidelberg University, Heidelberg, D-69120, Germanyen
local.contributor.departmentDepartment of Materials Science and Engineering, Uppsala University, Box 35, Uppsala, SE-751 03, Swedenen
local.contributor.departmentNational University of Science and Technology MISiS, Moscow, 119049, Russian Federationen
local.contributor.departmentLomonosov Moscow State University, Moscow, 119991, Russian Federationen
local.contributor.departmentUral Federal University, Ekaterinburg, 620002, Russian Federationen
local.contributor.departmentSchool of Science and Technology, Örebro University, Örebro, SE-701 82, Swedenen
local.contributor.departmentUniversity of Doha for Science and Technology, P.O. Box 24449, Doha, Qataren
local.identifier.pure37142201-
local.description.order115148-
local.identifier.eid2-s2.0-85151298553-
local.identifier.wosWOS:000961165700008-
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