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dc.contributor.authorBadrtdinov, D. I.en
dc.contributor.authorDing, L.en
dc.contributor.authorRitter, C.en
dc.contributor.authorHembacher, J.en
dc.contributor.authorAhmed, N.en
dc.contributor.authorSkourski, Y.en
dc.contributor.authorTsirlin, A. A.en
dc.date.accessioned2022-10-19T05:22:35Z-
dc.date.available2022-10-19T05:22:35Z-
dc.date.issued2021-
dc.identifier.citationMoP3SiO11: A4d3 honeycomb antiferromagnet with disconnected octahedra / D. I. Badrtdinov, L. Ding, C. Ritter et al. // Physical Review B. — 2021. — Vol. 104. — Iss. 9. — A16.en
dc.identifier.issn24699950-
dc.identifier.otherhttps://www.scopus.com/inward/record.uri?eid=2-s2.0-85115365262&doi=10.1103%2fPhysRevB.104.094428&partnerID=40&md5=95db80a9c27cf4a7e98e5f4e6f7fae44link
dc.identifier.urihttp://elar.urfu.ru/handle/10995/118129-
dc.description.abstractWe report the crystal structure and magnetic behavior of the spin- silicophosphate studied by high-resolution synchrotron x-ray diffraction, neutron diffraction, thermodynamic measurements, and ab initio band-structure calculations. Our data revise the crystallographic symmetry of this compound and establish its rhombohedral space group () along with the geometrically perfect honeycomb lattice of the ions residing in disconnected octahedra. Long-range antiferromagnetic order with the propagation vector observed below  K is a combined effect of the nearest-neighbor in-plane exchange coupling  K, easy-plane single-ion anisotropy  K, and a weak interlayer coupling  K. The 12% reduction in the ordered magnetic moment of the ions and the magnon gap of  K induced by the single-ion anisotropy further illustrate the impact of spin-orbit coupling on the magnetism. Our analysis puts forward single-ion anisotropy as an important ingredient of honeycomb antiferromagnets despite their nominally quenched orbital moment. ©2021 American Physical Societyen
dc.description.sponsorshipAlexander von Humboldt-Stiftung, AvH; Science and Technology Facilities Council, STFC; Deutsche Forschungsgemeinschaft, DFG: 107745057, TRR80; Bundesministerium für Bildung und Forschung, BMBF; Russian Science Foundation, RSF: 21-72-10136; Horizon 2020: 665593en
dc.description.sponsorshipWe are grateful to Anton Jesche for his continuous laboratory support and essential advice on thermodynamic measurements. The beam time provided by the ILL and ESRF was instrumental for completing this project. We thank Andy Fitch, Catherine Dejoie, and Vera Bader for their help during the data collection at ID22. We also acknowledge support by the HLD at HZDR, member of the European Magnetic Field Laboratory (EMFL).en
dc.description.sponsorshipRussian Science Foundation Alexander von Humboldt-Stiftung Deutsche Forschungsgemeinschaft Horizon 2020 Science and Technology Facilities Councilen
dc.format.mimetypeapplication/pdfen
dc.language.isoenen
dc.publisherAmerican Physical Societyen
dc.relationinfo:eu-repo/grantAgreement/RSF//21-72-10136en
dc.rightsinfo:eu-repo/semantics/openAccessen
dc.sourcePhysical Review Ben
dc.subjectANISOTROPYen
dc.subjectANTIFERROMAGNETIC MATERIALSen
dc.subjectCALCULATIONSen
dc.subjectCRYSTAL STRUCTUREen
dc.subjectION EXCHANGEen
dc.subjectIONSen
dc.subjectMAGNETIC MOMENTSen
dc.subjectNEUTRON DIFFRACTIONen
dc.subjectA: HONEYCOMBen
dc.subjectANTIFERROMAGNETSen
dc.subjectCRYSTALS STRUCTURESen
dc.subjectHIGH RESOLUTIONen
dc.subjectMAGNETIC BEHAVIORen
dc.subjectSILICOPHOSPHATESen
dc.subjectSINGLE ION ANISOTROPYen
dc.subjectSTRUCTURE BEHAVIORen
dc.subjectSYNCHROTRON X-RAY-DIFFRACTIONen
dc.subjectTHERMODYNAMIC MEASUREMENTSen
dc.subjectHONEYCOMB STRUCTURESen
dc.titleMoP3SiO11: A4d3 honeycomb antiferromagnet with disconnected octahedraen
dc.typeArticleen
dc.typeinfo:eu-repo/semantics/articleen
dc.typeinfo:eu-repo/semantics/publishedVersionen
dc.identifier.rsi47014135-
dc.identifier.doi10.1103/PhysRevB.104.094428-
dc.identifier.scopus85115365262-
local.contributor.employeeBadrtdinov, D.I., Theoretical Physics and Applied Mathematics Department, Ural Federal University, Yekaterinburg, 620002, Russian Federationen
local.contributor.employeeDing, L., ISIS Facility, Rutherford Appleton Laboratory, Harwell Oxford, Didcot, United Kingdom, Institut Néel, CNRS, Université, Joseph Fourier, Grenoble, 38042, Franceen
local.contributor.employeeRitter, C., Institut Laue-Langevin, BP 156, Grenoble, F-38042, Franceen
local.contributor.employeeHembacher, J., Experimental Physics VI, Center for Electronic Correlations and Magnetism, Institute of Physics, University of Augsburg, Augsburg, 86135, Germanyen
local.contributor.employeeAhmed, N., Experimental Physics VI, Center for Electronic Correlations and Magnetism, Institute of Physics, University of Augsburg, Augsburg, 86135, Germany, School of Physics, Indian Institute of Science Education and Research, Thiruvananthapuram, 695551, Indiaen
local.contributor.employeeSkourski, Y., Dresden High Magnetic Field Laboratory (HLD-EMFL), Helmholtz-Zentrum Dresden-Rossendorf, Dresden, 01328, Germanyen
local.contributor.employeeTsirlin, A.A., Theoretical Physics and Applied Mathematics Department, Ural Federal University, Yekaterinburg, 620002, Russian Federation, Experimental Physics VI, Center for Electronic Correlations and Magnetism, Institute of Physics, University of Augsburg, Augsburg, 86135, Germanyen
local.issue9-
local.volume104-
dc.identifier.wos000704237500002-
local.contributor.departmentTheoretical Physics and Applied Mathematics Department, Ural Federal University, Yekaterinburg, 620002, Russian Federationen
local.contributor.departmentISIS Facility, Rutherford Appleton Laboratory, Harwell Oxford, Didcot, United Kingdomen
local.contributor.departmentInstitut Néel, CNRS, Université, Joseph Fourier, Grenoble, 38042, Franceen
local.contributor.departmentInstitut Laue-Langevin, BP 156, Grenoble, F-38042, Franceen
local.contributor.departmentExperimental Physics VI, Center for Electronic Correlations and Magnetism, Institute of Physics, University of Augsburg, Augsburg, 86135, Germanyen
local.contributor.departmentSchool of Physics, Indian Institute of Science Education and Research, Thiruvananthapuram, 695551, Indiaen
local.contributor.departmentDresden High Magnetic Field Laboratory (HLD-EMFL), Helmholtz-Zentrum Dresden-Rossendorf, Dresden, 01328, Germanyen
local.identifier.pure23726698-
local.description.orderA16-
local.identifier.eid2-s2.0-85115365262-
local.fund.rsf21-72-10136-
local.identifier.wosWOS:000704237500002-
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