Пожалуйста, используйте этот идентификатор, чтобы цитировать или ссылаться на этот ресурс:
http://elar.urfu.ru/handle/10995/117835
Полная запись метаданных
Поле DC | Значение | Язык |
---|---|---|
dc.contributor.author | Politano, A. | en |
dc.contributor.author | Chiarello, G. | en |
dc.contributor.author | Kuo, C. -N. | en |
dc.contributor.author | Lue, C. S. | en |
dc.contributor.author | Edla, R. | en |
dc.contributor.author | Torelli, P. | en |
dc.contributor.author | Pellegrini, V. | en |
dc.contributor.author | Boukhvalov, D. W. | en |
dc.date.accessioned | 2022-10-19T05:19:47Z | - |
dc.date.available | 2022-10-19T05:19:47Z | - |
dc.date.issued | 2018 | - |
dc.identifier.citation | Tailoring the Surface Chemical Reactivity of Transition-Metal Dichalcogenide PtTe2 Crystals / A. Politano, G. Chiarello, C. -N. Kuo et al. // Advanced Functional Materials. — 2018. — Vol. 28. — Iss. 15. — 1706504. | en |
dc.identifier.issn | 1616301X | - |
dc.identifier.other | https://www.scopus.com/inward/record.uri?eid=2-s2.0-85041697938&doi=10.1002%2fadfm.201706504&partnerID=40&md5=0bb243698fea9c256a27ad873ab1ad07 | link |
dc.identifier.uri | http://elar.urfu.ru/handle/10995/117835 | - |
dc.description.abstract | PtTe2 is a novel transition-metal dichalcogenide hosting type-II Dirac fermions that displays application capabilities in optoelectronics and hydrogen evolution reaction. Here it is shown, by combining surface science experiments and density functional theory, that the pristine surface of PtTe2 is chemically inert toward the most common ambient gases (oxygen and water) and even in air. It is demonstrated that the creation of Te vacancies leads to the appearance of tellurium-oxide phases upon exposing defected PtTe2 surfaces to oxygen or ambient atmosphere, which is detrimental for the ambient stability of uncapped PtTe2-based devices. On the contrary, in PtTe2 surfaces modified by the joint presence of Te vacancies and substitutional carbon atoms, the stable adsorption of hydroxyl groups is observed, an essential step for water splitting and the water–gas shift reaction. These results thus pave the way toward the exploitation of this class of Dirac materials in catalysis. © 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim | en |
dc.description.sponsorship | Horizon 2020 Framework Programme, H2020: 696656-GrapheneCore1 | en |
dc.description.sponsorship | A.P. and G.C. thank Vito Fabio for technical support and Marilena Zappia for having participated in HREELS experiments. This work was partly performed in the framework of the Nanoscience Foundry and Fine Analysis (NFFA-MIUR Italy Progetti Internazionali) project under Proposal No. 2017004. This project received funding from the European Union’s Horizon 2020 research and innovation program under Grant Agreement No. 696656-GrapheneCore1. | en |
dc.format.mimetype | application/pdf | en |
dc.language.iso | en | en |
dc.publisher | Wiley-VCH Verlag | en |
dc.rights | info:eu-repo/semantics/openAccess | en |
dc.source | Advanced Functional Materials | en |
dc.subject | DENSITY FUNCTIONAL THEORY | en |
dc.subject | SURFACE SCIENCE | en |
dc.subject | TRANSITION-METAL DICHALCOGENIDES | en |
dc.subject | VIBRATIONAL SPECTROSCOPY | en |
dc.subject | X-RAY PHOTOELECTRON SPECTROSCOPY | en |
dc.subject | CARBON | en |
dc.subject | CHEMICAL SHIFT | en |
dc.subject | CHROMIUM COMPOUNDS | en |
dc.subject | DENSITY FUNCTIONAL THEORY | en |
dc.subject | DENSITY OF GASES | en |
dc.subject | TELLURIUM COMPOUNDS | en |
dc.subject | TRANSITION METALS | en |
dc.subject | VIBRATIONAL SPECTROSCOPY | en |
dc.subject | WATER GAS SHIFT | en |
dc.subject | X RAY PHOTOELECTRON SPECTROSCOPY | en |
dc.subject | AMBIENT ATMOSPHERE | en |
dc.subject | APPLICATION CAPABILITY | en |
dc.subject | HYDROGEN EVOLUTION REACTIONS | en |
dc.subject | PRISTINE SURFACES | en |
dc.subject | SURFACE CHEMICAL REACTIVITY | en |
dc.subject | SURFACE SCIENCE | en |
dc.subject | TRANSITION METAL DICHALCOGENIDES | en |
dc.subject | WATER GAS SHIFT (WGS) REACTION | en |
dc.subject | PLATINUM COMPOUNDS | en |
dc.title | Tailoring the Surface Chemical Reactivity of Transition-Metal Dichalcogenide PtTe2 Crystals | en |
dc.type | Article | en |
dc.type | info:eu-repo/semantics/article | en |
dc.type | info:eu-repo/semantics/publishedVersion | en |
dc.identifier.rsi | 35484443 | - |
dc.identifier.doi | 10.1002/adfm.201706504 | - |
dc.identifier.scopus | 85041697938 | - |
local.contributor.employee | Politano, A., Fondazione Istituto Italiano di Tecnologia, Graphene Labs, via Morego 30, Genova, 16163, Italy | en |
local.contributor.employee | Chiarello, G., Dipartimento di Fisica, Università della Calabria, via ponte Bucci cubo 31/C, Rende, Cosenza, 87036, Italy | en |
local.contributor.employee | Kuo, C.-N., Department of Physics, National Cheng Kung University, 1 Ta-Hsueh Road, Tainan, 70101, Taiwan | en |
local.contributor.employee | Lue, C.S., Department of Physics, National Cheng Kung University, 1 Ta-Hsueh Road, Tainan, 70101, Taiwan | en |
local.contributor.employee | Edla, R., Consiglio Nazionale delle Ricerche (CNR), Istituto Officina dei Materiali (IOM), Laboratorio TASC, Area Science Park, S.S. 14, km 163.5, Trieste, 34149, Italy | en |
local.contributor.employee | Torelli, P., Consiglio Nazionale delle Ricerche (CNR), Istituto Officina dei Materiali (IOM), Laboratorio TASC, Area Science Park, S.S. 14, km 163.5, Trieste, 34149, Italy | en |
local.contributor.employee | Pellegrini, V., Fondazione Istituto Italiano di Tecnologia, Graphene Labs, via Morego 30, Genova, 16163, Italy | en |
local.contributor.employee | Boukhvalov, D.W., Department of Chemistry, Haiyang University, 17 Haengdang-dong, Seongdong-gu, Seoul, 04763, South Korea, Theoretical Physics and Applied Mathematics Department, Ural Federal University, Mira Street 19, Ekaterinburg, 620002, Russian Federation | en |
local.issue | 15 | - |
local.volume | 28 | - |
dc.identifier.wos | 000430101100020 | - |
local.contributor.department | Fondazione Istituto Italiano di Tecnologia, Graphene Labs, via Morego 30, Genova, 16163, Italy | en |
local.contributor.department | Dipartimento di Fisica, Università della Calabria, via ponte Bucci cubo 31/C, Rende, Cosenza, 87036, Italy | en |
local.contributor.department | Department of Physics, National Cheng Kung University, 1 Ta-Hsueh Road, Tainan, 70101, Taiwan | en |
local.contributor.department | Consiglio Nazionale delle Ricerche (CNR), Istituto Officina dei Materiali (IOM), Laboratorio TASC, Area Science Park, S.S. 14, km 163.5, Trieste, 34149, Italy | en |
local.contributor.department | Department of Chemistry, Haiyang University, 17 Haengdang-dong, Seongdong-gu, Seoul, 04763, South Korea | en |
local.contributor.department | Theoretical Physics and Applied Mathematics Department, Ural Federal University, Mira Street 19, Ekaterinburg, 620002, Russian Federation | en |
local.identifier.pure | 7146732 | - |
local.description.order | 1706504 | - |
local.identifier.eid | 2-s2.0-85041697938 | - |
local.identifier.wos | WOS:000430101100020 | - |
Располагается в коллекциях: | Научные публикации ученых УрФУ, проиндексированные в SCOPUS и WoS CC |
Файлы этого ресурса:
Файл | Описание | Размер | Формат | |
---|---|---|---|---|
2-s2.0-85041697938.pdf | 639,41 kB | Adobe PDF | Просмотреть/Открыть |
Все ресурсы в архиве электронных ресурсов защищены авторским правом, все права сохранены.