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dc.contributor.authorD’olimpio, G.en
dc.contributor.authorZhang, L.en
dc.contributor.authorKuo, C. -N.en
dc.contributor.authorFarias, D.en
dc.contributor.authorOttaviano, L.en
dc.contributor.authorLue, C. S.en
dc.contributor.authorFujii, J.en
dc.contributor.authorVobornik, I.en
dc.contributor.authorAgarwal, A.en
dc.contributor.authorTorelli, P.en
dc.contributor.authorBoukhvalov, D. W.en
dc.contributor.authorPolitano, A.en
dc.date.accessioned2022-05-12T08:30:51Z-
dc.date.available2022-05-12T08:30:51Z-
dc.date.issued2022-
dc.identifier.citationEfficient Hydrogen Evolution Reaction with Bulk and Nanostructured Mitrofanovite Pt3 Te4 / G. D’olimpio, L. Zhang, C. -N. Kuo et al. // Nanomaterials. — 2022. — Vol. 12. — Iss. 3. — 558.en
dc.identifier.issn2079-4991-
dc.identifier.otherAll Open Access, Gold, Green3
dc.identifier.urihttp://elar.urfu.ru/handle/10995/112223-
dc.description.abstractHere, we discuss the key features of electrocatalysis with mitrofanovite (Pt3 Te4 ), a recently discovered mineral with superb performances in hydrogen evolution reaction. Mitrofanovite is a layered topological metal with spin-polarized topological surface states with potential applications for spintronics. However, mitrofanovite is also an exceptional platform for electrocatalysis, with costs of the electrodes suppressed by 47% owing to the partial replacement of Pt with Te. Remarkably, the Tafel slope in nanostructured mitrofanovite is just 33 mV/dec, while reduced mitrofanovite has the same Tafel slope (36 mV/dec) as state-of-the-art electrodes of pure Pt. Mitrofanovite also affords surface stability and robustness to CO poisoning. Accordingly, these findings pave the way for the advent of mitrofanovite for large-scale hydrogen production. © 2022 by the authors. Licensee MDPI, Basel, Switzerland.en
dc.description.sponsorshipFunding: D.W.B. acknowledges support from the Ministry of Science and Higher Education of the Russian Federation (through the basic part of the government mandate, Project No. FEUZ-2020– 0060) and the Jiangsu Innovative and Entrepreneurial Talents Project. This work has been partially supported by the Spanish Ministerio de Ciencia e Innovación under Project PID2019–109525RB-I00. D.F. acknowledges financial support from the Spanish Ministry of Economy and Competitiveness, through the “Maríade Maeztu” Programme for Units of Excellence in R&D (CEX2018-000805-M). I.V., J. F., and P.T. thank NFFA-Trieste.en
dc.format.mimetypeapplication/pdfen
dc.language.isoenen
dc.publisherMDPIen1
dc.publisherMDPI AGen
dc.rightsinfo:eu-repo/semantics/openAccessen
dc.sourceNanomaterials2
dc.sourceNanomaterialsen
dc.subjectELECTROCATALYSISen
dc.subjectHYDROGEN EVOLUTION REACTIONen
dc.subjectMETAL CHALCOGENIDESen
dc.titleEfficient Hydrogen Evolution Reaction with Bulk and Nanostructured Mitrofanovite Pt3 Te4en
dc.typeArticleen
dc.typeinfo:eu-repo/semantics/articleen
dc.typeinfo:eu-repo/semantics/publishedVersionen
dc.identifier.doi10.3390/nano12030558-
dc.identifier.scopus85123945901-
local.contributor.employeeD’olimpio, G., Department of Physical and Chemical Sciences, University of L’Aquila, Via Vetoio, L’Aquila, 67100, Italy; Zhang, L., College of Chemistry and Chemical Engineering, Qingdao University, Qingdao, 266071, China; Kuo, C.-N., Department of Physics, National Cheng Kung University, 1 Ta-Hsueh Road, Tainan, 70101, Taiwan, Taiwan Consortium of Emergent Crystalline Materials, Ministry of Science and Technology, Taipei, 10601, Taiwan; Farias, D., Departamento de Física de la Materia Condensada, Universidad Autónoma de Madrid, Madrid, 28049, Spain, Instituto “Nicolás Cabrera”, Campus de Cantoblanco, Madrid, 28049, Spain, Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, Madrid, 28049, Spain; Ottaviano, L., Department of Physical and Chemical Sciences, University of L’Aquila, Via Vetoio, L’Aquila, 67100, Italy, CNR-SPIN, Uos L’Aquila, Via Vetoio 10, L’Aquila, 67100, Italy; Lue, C.S., Department of Physics, National Cheng Kung University, 1 Ta-Hsueh Road, Tainan, 70101, Taiwan, Taiwan Consortium of Emergent Crystalline Materials, Ministry of Science and Technology, Taipei, 10601, Taiwan; Fujii, J., CNR-IOM, TASC Laboratory, Area Science Park-Basovizza, Trieste, 34149, Italy; Vobornik, I., CNR-IOM, TASC Laboratory, Area Science Park-Basovizza, Trieste, 34149, Italy; Agarwal, A., Department of Physics, Indian Institute of Technology Kanpur, Kanpur, 208016, India; Torelli, P., CNR-IOM, TASC Laboratory, Area Science Park-Basovizza, Trieste, 34149, Italy; Boukhvalov, D.W., College of Science, Institute of Materials Physics and Chemistry, Nanjing Forestry University, Nanjing, 210037, China, Theoretical Physics and Applied Mathematics Department, Ural Federal University, Mira Street 19, Ekaterinburg, 620002, Russian Federation; Politano, A., Department of Physical and Chemical Sciences, University of L’Aquila, Via Vetoio, L’Aquila, 67100, Italy, CNR-IMM, Istituto per la Microelettronica e Microsistemi, VIII Strada 5, Catania, 95121, Italy, INSTM, University of L’Aquila Unit, L’Aquila, 67100, Italyen
local.issue3-
local.volume12-
dc.identifier.wos000757542100001-
local.contributor.departmentDepartment of Physical and Chemical Sciences, University of L’Aquila, Via Vetoio, L’Aquila, 67100, Italy; College of Chemistry and Chemical Engineering, Qingdao University, Qingdao, 266071, China; Department of Physics, National Cheng Kung University, 1 Ta-Hsueh Road, Tainan, 70101, Taiwan; Taiwan Consortium of Emergent Crystalline Materials, Ministry of Science and Technology, Taipei, 10601, Taiwan; Departamento de Física de la Materia Condensada, Universidad Autónoma de Madrid, Madrid, 28049, Spain; Instituto “Nicolás Cabrera”, Campus de Cantoblanco, Madrid, 28049, Spain; Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, Madrid, 28049, Spain; CNR-SPIN, Uos L’Aquila, Via Vetoio 10, L’Aquila, 67100, Italy; CNR-IOM, TASC Laboratory, Area Science Park-Basovizza, Trieste, 34149, Italy; Department of Physics, Indian Institute of Technology Kanpur, Kanpur, 208016, India; College of Science, Institute of Materials Physics and Chemistry, Nanjing Forestry University, Nanjing, 210037, China; Theoretical Physics and Applied Mathematics Department, Ural Federal University, Mira Street 19, Ekaterinburg, 620002, Russian Federation; CNR-IMM, Istituto per la Microelettronica e Microsistemi, VIII Strada 5, Catania, 95121, Italy; INSTM, University of L’Aquila Unit, L’Aquila, 67100, Italyen
local.identifier.pure29558783-
local.description.order558-
local.identifier.eid2-s2.0-85123945901-
local.identifier.wosWOS:000757542100001-
local.fund.feuzFEUZ-2020- 0060-
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