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dc.contributor.authorKorzhik, M.en
dc.contributor.authorRetivov, V.en
dc.contributor.authorBondarau, A.en
dc.contributor.authorDosovitskiy, G.en
dc.contributor.authorDubov, V.en
dc.contributor.authorKamenskikh, I.en
dc.contributor.authorKarpuk, P.en
dc.contributor.authorKuznetsova, D.en
dc.contributor.authorSmyslova, V.en
dc.contributor.authorMechinsky, V.en
dc.contributor.authorPustovarov, V.en
dc.contributor.authorTavrunov, D.en
dc.contributor.authorTishchenko, E.en
dc.contributor.authorVasil’ev, A.en
dc.date.accessioned2024-04-08T11:08:04Z-
dc.date.available2024-04-08T11:08:04Z-
dc.date.issued2022-
dc.identifier.citationKorzhik, M, Retivov, V, Bondarau, A, Dosovitskiy, G, Dubov, V, Kamenskikh, I, Karpuk, P, Kuznetsova, D, Smyslova, V, Mechinsky, V, Pustovarov, V, Tavrunov, D, Tishchenko, E & Vasil’ev, A 2022, 'Role of the Dilution of the Gd Sublattice in Forming the Scintillation Properties of Quaternary (Gd,Lu)3Al2Ga3O12: Ce Ceramics', Crystals, Том. 12, № 9, 1196, стр. 1196. https://doi.org/10.3390/cryst12091196harvard_pure
dc.identifier.citationKorzhik, M., Retivov, V., Bondarau, A., Dosovitskiy, G., Dubov, V., Kamenskikh, I., Karpuk, P., Kuznetsova, D., Smyslova, V., Mechinsky, V., Pustovarov, V., Tavrunov, D., Tishchenko, E., & Vasil’ev, A. (2022). Role of the Dilution of the Gd Sublattice in Forming the Scintillation Properties of Quaternary (Gd,Lu)3Al2Ga3O12: Ce Ceramics. Crystals, 12(9), 1196. [1196]. https://doi.org/10.3390/cryst12091196apa_pure
dc.identifier.issn2073-4352-
dc.identifier.otherFinal2
dc.identifier.otherAll Open Access; Gold Open Access3
dc.identifier.otherhttps://www.mdpi.com/2073-4352/12/9/1196/pdf?version=16615086591
dc.identifier.otherhttps://www.mdpi.com/2073-4352/12/9/1196/pdf?version=1661508659pdf
dc.identifier.urihttp://elar.urfu.ru/handle/10995/131567-
dc.description.abstractTechnological factors and processes contributing to the scintillation mechanism have been considered in quaternary garnet ceramics doped with Ce(Gd,Lu)3Al2Ga3O12. The super-stoichiometric additive of gadolinium in the material composition or its co-doping with a low concentration of Mg were found to be effective tools to suppress phosphorescence in the quaternary garnet, confirming that it is not an intrinsic property of the material. The Monte-Carlo simulation of electronic excitation transfer demonstrates that the hopping migration along the gadolinium sublattice plays an essential role in forming the scintillation kinetic parameters. Breaking the integrity of the gadolinium sublattice by substitution with heavier lutetium ions increases the role of self-trapped states in the excitation of Ce3+ ions, which ensures both an increase in the fraction of short ~20 ns and very long ~600 ns components in the scintillation kinetics. © 2022 by the authors.en
dc.description.sponsorshipIREAen
dc.description.sponsorshipNational Research Council Canada, NRCen
dc.description.sponsorshipMinistry of Education and Science of the Russian Federation, Minobrnauka, (075-15-2021-1353, FEUZ-2020-0060)en
dc.description.sponsorshipRussian Science Foundation, RSF, (21-12-00219)en
dc.description.sponsorshipMinistry of Science and Higher Education of the Russian Federation, (075-11-2021-070)en
dc.description.sponsorshipMidlands State University, MSUen
dc.description.sponsorshipAuthors from NRC “Kurchatov Institute” and MSU acknowledge support from the Russian Ministry of Science and Education through grant No. 075-15-2021-1353. The access to the scientific equipment at shared research facilities at the Scientific Research Analytical Center of National Research Center “Kurchatov Institute”—IREA, with financial support by the Russian Ministry of Science and Higher Education (agreement no. 075-11-2021-070 of 19/08/2021) is also appreciated. The research at Ural Federal University was partially supported by the Ministry of Science and Higher Education of the Russian Federation (project FEUZ-2020-0060). The Monte-Carlo simulation of the migration was supported by the Russian Scientific Fund, grant 21-12-00219.en
dc.format.mimetypeapplication/pdfen
dc.language.isoenen
dc.publisherMDPIen
dc.relationinfo:eu-repo/grantAgreement/RSF//21-12-00219en
dc.rightsinfo:eu-repo/semantics/openAccessen
dc.rightscc-byother
dc.rights.urihttps://creativecommons.org/licenses/by/4.0/unpaywall
dc.sourceCrystals2
dc.sourceCrystalsen
dc.subjectCERIUMen
dc.subjectDECAY TIMEen
dc.subjectLIGHT YIELDen
dc.subjectLUTETIUMen
dc.subjectPHOSPHORESCENCEen
dc.subjectQUATERNARY GARNETen
dc.subjectSCINTILLATIONen
dc.titleRole of the Dilution of the Gd Sublattice in Forming the Scintillation Properties of Quaternary (Gd,Lu)3Al2Ga3O12: Ce Ceramicsen
dc.typeArticleen
dc.typeinfo:eu-repo/semantics/articleen
dc.typeinfo:eu-repo/semantics/publishedVersionen
dc.identifier.doi10.3390/cryst12091196-
dc.identifier.scopus85138621333-
local.contributor.employeeKorzhik M., Institute for Nuclear Problems, Belarus State University, 11 Bobruiskaya, Minsk, 220030, Belarus, National Research Center “Kurchatov Institute”, Moscow, 123098, Russian Federationen
local.contributor.employeeRetivov V., National Research Center “Kurchatov Institute”, Moscow, 123098, Russian Federation, NRC “Kurchatov Institute”—IREA, Moscow, 107076, Russian Federationen
local.contributor.employeeBondarau A., Institute for Nuclear Problems, Belarus State University, 11 Bobruiskaya, Minsk, 220030, Belarusen
local.contributor.employeeDosovitskiy G., NRC “Kurchatov Institute”—IREA, Moscow, 107076, Russian Federationen
local.contributor.employeeDubov V., National Research Center “Kurchatov Institute”, Moscow, 123098, Russian Federation, NRC “Kurchatov Institute”—IREA, Moscow, 107076, Russian Federationen
local.contributor.employeeKamenskikh I., Physical Department of Moscow State University, Moscow, 119991, Russian Federationen
local.contributor.employeeKarpuk P., National Research Center “Kurchatov Institute”, Moscow, 123098, Russian Federation, NRC “Kurchatov Institute”—IREA, Moscow, 107076, Russian Federationen
local.contributor.employeeKuznetsova D., National Research Center “Kurchatov Institute”, Moscow, 123098, Russian Federation, NRC “Kurchatov Institute”—IREA, Moscow, 107076, Russian Federationen
local.contributor.employeeSmyslova V., National Research Center “Kurchatov Institute”, Moscow, 123098, Russian Federation, NRC “Kurchatov Institute”—IREA, Moscow, 107076, Russian Federationen
local.contributor.employeeMechinsky V., Institute for Nuclear Problems, Belarus State University, 11 Bobruiskaya, Minsk, 220030, Belarus, National Research Center “Kurchatov Institute”, Moscow, 123098, Russian Federationen
local.contributor.employeePustovarov V., Physics Department, Ural Federal University, Yekaterinburg, 620002, Russian Federationen
local.contributor.employeeTavrunov D., Physics Department, Ural Federal University, Yekaterinburg, 620002, Russian Federationen
local.contributor.employeeTishchenko E., Physical Department of Moscow State University, Moscow, 119991, Russian Federationen
local.contributor.employeeVasil’ev A., Skobelchin Institute for Nuclear Physics, Moscow State University, Moscow, 119991, Russian Federationen
local.issue9-
local.volume12-
dc.identifier.wos000856335400001-
local.contributor.departmentInstitute for Nuclear Problems, Belarus State University, 11 Bobruiskaya, Minsk, 220030, Belarusen
local.contributor.departmentNational Research Center “Kurchatov Institute”, Moscow, 123098, Russian Federationen
local.contributor.departmentNRC “Kurchatov Institute”—IREA, Moscow, 107076, Russian Federationen
local.contributor.departmentPhysical Department of Moscow State University, Moscow, 119991, Russian Federationen
local.contributor.departmentPhysics Department, Ural Federal University, Yekaterinburg, 620002, Russian Federationen
local.contributor.departmentSkobelchin Institute for Nuclear Physics, Moscow State University, Moscow, 119991, Russian Federationen
local.identifier.pure30944847-
local.identifier.pureea06cd6a-546b-4f64-bb03-288127b33c39uuid
local.description.order1196-
local.identifier.eid2-s2.0-85138621333-
local.fund.rsf21-12-00219-
local.identifier.wosWOS:000856335400001-
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