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dc.contributor.authorZhitkov, A.en
dc.contributor.authorPotapov, A.en
dc.contributor.authorKarimov, K.en
dc.contributor.authorKholkina, A.en
dc.contributor.authorShishkin, V.en
dc.contributor.authorDedyukhin, A.en
dc.contributor.authorZaykov, Y.en
dc.date.accessioned2022-05-12T08:31:12Z-
dc.date.available2022-05-12T08:31:12Z-
dc.date.issued2022-
dc.identifier.citationInteraction between UN and CdCl2 in Molten LiCl–KCl Eutectic. II. Experiment at 1023 K / A. Zhitkov, A. Potapov, K. Karimov et al. // Nuclear Engineering and Technology. — 2022. — Vol. 54. — Iss. 2. — P. 653-660.en
dc.identifier.issn1738-5733-
dc.identifier.otherAll Open Access, Gold3
dc.identifier.urihttp://elar.urfu.ru/handle/10995/112247-
dc.description.abstractThe interaction between UN and CdCl2 in the LiCl–KCl molten eutectic was studied at 1023 K. The chlorination was monitored by sampling and recording the redox potential of the medium. At 1023 K the chlorination of UN with cadmium chloride in the molten LiCl–KCl eutectic proceeds completely and results in the formation of uranium chlorides. The melts of the LiCl–KCl–UCl3 or LiCl–KCl–UCl4 compositions can be obtained by the end of experiment depending on the presence of metallic cadmium in the reaction zone. The higher the concentration of the chlorinating agent, the faster the reaction rate. At [CdCl2]/[UN] = 1.65 (10% excess) the reaction proceeds to completion in about 7.5 h. At [CdCl2]/[UN] = 7 the complete chlorination takes 2.5–3 h. © 2021.en
dc.description.sponsorshipThe authors gratefully acknowledge for analytical support of the Shared Access Centre "Composition of Compounds" of the Institute of High Temperature Electrochemistry of the Ural Branch of the Russian Academy of Sciences. The present research was partially performed within the Proryv (Breakthrough) project of State Atomic Energy Corporation Rosatom.en
dc.format.mimetypeapplication/pdfen
dc.language.isoenen
dc.publisherKorean Nuclear Societyen1
dc.publisherElsevier BVen
dc.rightsinfo:eu-repo/semantics/openAccessen
dc.sourceNucl. Eng. Technol.2
dc.sourceNuclear Engineering and Technologyen
dc.subjectCDCL2en
dc.subjectCHLORINATIONen
dc.subjectMOLTEN SALTSen
dc.subjectNITRIDE NUCLEAR FUELen
dc.subjectPYROCHEMISTRYen
dc.subjectREPROCESSING OF SPENT NUCLEAR FUELen
dc.subjectUNen
dc.titleInteraction between UN and CdCl2 in Molten LiCl–KCl Eutectic. II. Experiment at 1023 Ken
dc.typeArticleen
dc.typeinfo:eu-repo/semantics/articleen
dc.typeinfo:eu-repo/semantics/publishedVersionen
dc.identifier.rsi47054636-
dc.identifier.doi10.1016/j.net.2021.08.030-
dc.identifier.scopus85114692231-
local.contributor.employeeZhitkov, A., Institute of High Temperature Electrochemistry of the Ural Branch of the Russian Academy of Sciences, Akademicheskaya Str. 20, Ekaterinburg, Russian Federation; Potapov, A., Institute of High Temperature Electrochemistry of the Ural Branch of the Russian Academy of Sciences, Akademicheskaya Str. 20, Ekaterinburg, Russian Federation, Ural State Mining University, Ekaterinburg, Russian Federation; Karimov, K., Institute of High Temperature Electrochemistry of the Ural Branch of the Russian Academy of Sciences, Akademicheskaya Str. 20, Ekaterinburg, Russian Federation; Kholkina, A., Institute of High Temperature Electrochemistry of the Ural Branch of the Russian Academy of Sciences, Akademicheskaya Str. 20, Ekaterinburg, Russian Federation, Ural Federal University, Ekaterinburg, Russian Federation; Shishkin, V., Institute of High Temperature Electrochemistry of the Ural Branch of the Russian Academy of Sciences, Akademicheskaya Str. 20, Ekaterinburg, Russian Federation; Dedyukhin, A., Institute of High Temperature Electrochemistry of the Ural Branch of the Russian Academy of Sciences, Akademicheskaya Str. 20, Ekaterinburg, Russian Federation; Zaykov, Y., Institute of High Temperature Electrochemistry of the Ural Branch of the Russian Academy of Sciences, Akademicheskaya Str. 20, Ekaterinburg, Russian Federation, Ural Federal University, Ekaterinburg, Russian Federationen
local.description.firstpage653-
local.description.lastpage660-
local.issue2-
local.volume54-
dc.identifier.wos000752500200006-
local.contributor.departmentInstitute of High Temperature Electrochemistry of the Ural Branch of the Russian Academy of Sciences, Akademicheskaya Str. 20, Ekaterinburg, Russian Federation; Ural State Mining University, Ekaterinburg, Russian Federation; Ural Federal University, Ekaterinburg, Russian Federationen
local.identifier.pure29563389-
local.identifier.eid2-s2.0-85114692231-
local.identifier.wosWOS:000752500200006-
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